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Litter decomposition is a key process for carbon and nutrient cycling in terrestrial ecosystems and is mainly controlled by environmental conditions, substrate quantity and quality as well as microbial community abundance and composition. In particular, the effects of climate and atmospheric nitrogen (N) deposition on litter decomposition and its temporal dynamics are of significant importance, since their effects might change over the course of the decomposition process. Within the TeaComposition initiative, we incubated Green and Rooibos teas at 524 sites across nine biomes. We assessed how macroclimate and atmospheric inorganic N deposition under current and predicted scenarios (RCP 2.6, RCP 8.5) might affect litter mass loss measured after 3 and 12 months. Our study shows that the early to mid-term mass loss at the global scale was affected predominantly by litter quality (explaining 73% and 62% of the total variance after 3 and 12 months, respectively) followed by climate and N deposition. The effects of climate were not litter-specific and became increasingly significant as decomposition progressed, with MAP explaining 2% and MAT 4% of the variation after 12 months of incubation. The effect of N deposition was litter-specific, and significant only for 12-month decomposition of Rooibos tea at the global scale. However, in the temperate biome where atmospheric N deposition rates are relatively high, the 12-month mass loss of Green and Rooibos teas decreased significantly with increasing N deposition, explaining 9.5% and 1.1% of the variance, respectively. The expected changes in macroclimate and N deposition at the global scale by the end of this century are estimated to increase the 12-month mass loss of easily decomposable litter by 1.1–3.5% and of the more stable substrates by 3.8–10.6%, relative to current mass loss. In contrast, expected changes in atmospheric N deposition will decrease the mid-term mass loss of high-quality litter by 1.4–2.2% and that of low-quality litter by 0.9–1.5% in the temperate biome. Our results suggest that projected increases in N deposition may have the capacity to dampen the climate-driven increases in litter decomposition depending on the biome and decomposition stage of substrate. 

Abstract. For the radiative impact of individual climate forcings,most previous studies focused on the global mean values at the top of theatmosphere (TOA), and less attention has been paid to surface processes,especially for black carbon (BC) aerosols. In this study, the surface radiativeresponses to five different forcing agents were analyzed by using idealizedmodel simulations. Our analyses reveal that for greenhouse gases, solarirradiance, and scattering aerosols, the surface temperature changes aremainly dictated by the changes of surface radiative heating, but for BC,surface energy redistribution between different components plays a morecrucial role. Globally, when a unit BC forcing is imposed at TOA, the netshortwave radiation at the surface decreases by -5.87±0.67 W m−2 (W m−2)−1 (averaged over global land without Antarctica), which ispartially offset by increased downward longwave radiation (2.32±0.38 W m−2 (W m−2)−1 from the warmer atmosphere, causing a netdecrease in the incoming downward surface radiation of -3.56±0.60 W m−2 (W m−2)−1. Despite a reduction in the downward radiationenergy, the surface air temperature still increases by 0.25±0.08 Kbecause of less efficient energy dissipation, manifested by reduced surfacesensible (-2.88±0.43 W m−2 (W m−2)−1) and latent heat flux(-1.54±0.27 W m−2 (W m−2)−1), as well as a decrease inBowen ratio (-0.20±0.07 (W m−2)−1). Such reductions of turbulentfluxes can be largely explained by enhanced air stability (0.07±0.02 K (W m−2)−1), measured as the difference of the potential temperaturebetween 925 hPa and surface, and reduced surface wind speed (-0.05±0.01 m s−1 (W m−2)−1). The enhanced stability is due to the fasteratmospheric warming relative to the surface, whereas the reduced wind speedcan be partially explained by enhanced stability and reduced Equator-to-poleatmospheric temperature gradient. These rapid adjustments under BC forcingoccur in the lower atmosphere and propagate downward to influence thesurface energy redistribution and thus surface temperature response, whichis not observed under greenhouse gases or scattering aerosols. Our studyprovides new insights into the impact of absorbing aerosols on surfaceenergy balance and surface temperature response. 

Abstract Biomass burning aerosol (BBA) emissions in the Coupled Model Intercomparison Project phase 6 (CMIP6) historical forcing fields have enhanced temporal variability during the years 1997–2014 compared to earlier periods. Recent studies document that the corresponding inhomogeneous shortwave forcing over this period can cause changes in clouds, permafrost, and soil moisture, which contribute to a net terrestrial Northern Hemisphere warming relative to earlier periods. Here, we investigate the ocean response to the hemispherically asymmetric warming, using a 100-member ensemble of the Community Earth System Model version 2 Large Ensemble forced by two different BBA emissions (CMIP6 default and temporally smoothed over 1990–2020). Differences between the two subensemble means show that ocean temperature anomalies occur during periods of high BBA variability and subsequently persist over multiple decades. In the North Atlantic, surface warming is efficiently compensated for by decreased northward oceanic heat transport due to a slowdown of the Atlantic meridional overturning circulation. In the North Pacific, surface warming is compensated for by an anomalous cross-equatorial cell (CEC) that reduces northward oceanic heat transport. The heat that converges in the South Pacific through the anomalous CEC is shunted into the subsurface and contributes to formation of long-lasting ocean temperature anomalies. The anomalous CEC is maintained through latitude-dependent contributions from narrow western boundary currents and basinwide near-surface Ekman transport. These results indicate that interannual variability in forcing fields may significantly change the background climate state over long time scales, presenting a potential uncertainty in CMIP6-class climate projections forced without interannual variability.